物理化学学报ActaPhys.-Chim.Sin.2023,39(11),2301001(1of22)Received:January1,2023;Revised:February21,2023;Accepted:February21,2023;Publishedonline:March6,2023.*Correspondingauthors.Emails:qitao-zhang@szu.edu.cn(Q.Z.);chmsuc@szu.edu.cn(C.S.);Tel.:+86-15875517091(Q.Z.);+86-13066870440(C.S.).TheprojectwassupportedbytheNationalNaturalScienceFoundationofChina(21972094,21805191,22102102),NationalKeyResearchandDevelopmentProgramofChina(2021YFA1600800),EducationalCommissionofGuangdongProvince,China(839-0000013131),GuangdongBasicandAppliedBasicResearchFoundation,China(2020A1515010982),ShenzhenScienceandTechnologyProgram,China(JCYJ20190808142001745,RCJC20200714114434086),ShenzhenStableSupportProject,China(20200812160737002,20200812122947002),ShenzhenPeacockPlan,China(20180921273B,202108022524B,20210308299C).国家自然科学基金(21972094,21805191,22102102),国家重点研发计划(2021YFA1600800),广东省教育厅基金(839-0000013131),广东基础和应用基础研究基金(2020A1515010982),深圳科技计划(JCYJ2019080808142001745,RCJC2020200714114434086),深圳稳定支持项目(20200812160737002,20200812122947002),深圳孔雀计划(20180921273B,202108022524B,20210308299C)资助©EditorialofficeofActaPhysico-ChimicaSinica[Review]doi:10.3866/PKU.WHXB202301001www.whxb.pku.edu.cnSemiconductingPolymersforPhotosynthesisofH2O2:SpatialSeparationandSynergisticUtilizationofPhotoredoxCentersYaoXie1,QitaoZhang1,*,HongliSun1,ZhenyuanTeng2,3,ChenliangSu1,*1InternationalCollaborativeLaboratoryof2DMaterialsforOptoelectronicScience&Technology,EngineeringTechnologyResearchCenterfor2DMaterialsInformationFunctionalDevicesandSystemsofGuangdongProvince,InstituteofMicroscaleOptoeletronics,ShenzhenUniversity,Shenzhen518060,GuangdongProvince,China.2SchoolofChemistry,ChemicalEngineeringandBiotechnology,NanyangTechnologicalUniversity,Singapore637459,Singapore.3DepartmentofAppliedChemistry,FacultyofEngineering,KyushuInstituteofTechnology,Kitakyushu804-8550,Japan.Abstract:Thephotocatalyticsynthesisofhydrogenperoxideusingearth-abundantwaterand/or...